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Since the first report on the 9.7% efficient and 500 h-stable solid-state perovskite solar cell (PSC) in 2012, following two seed reports on perovskite-sensitized liquid junction solar cells in 2009 and 2011, research on perovskite photovoltaics has surged due to the high power conversion efficiency (PCE) obtainable via facile fabrication procedures. As a result, a PCE of 25.2% was recorded in 2019. According to Web of Science, the number of publications on PSCs has grown exponentially since 2012, leading to more than 15,500 accumulated papers, which indicates that PSCs are considered as promising next-generation photovoltaics. Over the past 10 years, high photovoltaic performance has been realized through compositional engineering, device architecture, and new coating methodologies. To reach a theoretical efficiency over 30% and commercialization of PSCs, further studies on recombination and developments of scalable technologies are required. In this talk, the importance of interfacial and grain boundary engineering to reach the theoretical efficiency with voltage over 1.3 V and fill factor over 0.9 is emphasized. For commercialization, new materials may be required because the current precursor mixture is problematic due to the underlying aging effect. We developed cost-effective materials based on delta FAPbI3 powder for reproducibly high efficiency PSCs. Large-area uniform perovskite coating is also important in upscaling PSCs. Acetonitrile-based and 2 methoxy ethanol-based coating solutions were developed for large-area perovskite films. In addition, additive engineering and bifacial stamping technique were found to be effective ways for upscaling PSCs. Stability is also discussed throughout the talk. Read "5 Questions with Dr. Nam-Gyu Park" for more insight on his talk, here: https://www.electrochem.org/ecs-blog/...